Double-resonant LA phonon scattering in defective graphene and carbon nanotubes

Herziger F, Tyborski C, Ochedowski O, Schleberger M, Maultzsch J (2014)

Publication Status: Published

Publication Type: Journal article

Publication year: 2014

Journal

Physical Review B American Physical Society

Publisher: AMER PHYSICAL SOC

Book Volume: 90

Journal Issue: 24

DOI: 10.1103/PhysRevB.90.245431

Open Access Link: https://arxiv.org/abs/1412.4501

Abstract

We present measurements of the D '' Raman mode in graphene and carbon nanotubes at different laser excitation energies. The Raman mode around 1050-1150 cm(-1) originates from a double-resonant scattering process of longitudinal acoustic (LA) phonons with defects. We investigate its dependence on laser excitation energy, on the number of graphene layers, and on the carbon nanotube diameter. We assign this Raman mode to so-called inner processes with resonant phonons mainly from the Gamma-K high-symmetry direction. The asymmetry of the D '' mode is explained by additional contributions from phonons next to the Gamma-K line. Our results demonstrate the importance of inner contributions in the double-resonance scattering process and add a fast method to investigate acoustic phonons in graphene and carbon nanotubes by optical spectroscopy.

Authors with CRIS profile

Janina Maultzsch Lehrstuhl für Experimentalphysik

Involved external institutions

Technische Universität Berlin DE Germany (DE) Universität Duisburg-Essen (UDE) DE Germany (DE)

How to cite

APA:

Herziger, F., Tyborski, C., Ochedowski, O., Schleberger, M., & Maultzsch, J. (2014). Double-resonant LA phonon scattering in defective graphene and carbon nanotubes. Physical Review B, 90(24). https://doi.org/10.1103/PhysRevB.90.245431

MLA:

Herziger, Felix, et al. "Double-resonant LA phonon scattering in defective graphene and carbon nanotubes." Physical Review B 90.24 (2014).

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