Hanus V, Kangaparambil S, Richter M, Hassfurth L, Dorner-Kirchner M, Paulus GG, Xie X, Baltuska A, Gräfe S, Zeiler M (2023)
Publication Type: Journal article
Publication year: 2023
Book Volume: 25
Pages Range: 4656-4666
Journal Issue: 6
DOI: 10.1039/d2cp03077b
We report on a combined experimental and numerical study of photoelectron circular dichroism (PECD) induced by intense few-cycle laser pulses, using methyloxirane as the molecular example. Our experiments reveal a remarkably pronounced sensitivity of the PECD strength of double-ionization on the carrier-envelope phase (CEP) of the laser pulses. By comparison to the simulations, which reproduce the measured CEP-dependence for specific orientations of the molecules in the lab frame, we attribute the origin of the observed CEP-dependence of PECD to the CEP-induced modulation of ionization from different areas of the wave functions of three dominant orbitals.
APA:
Hanus, V., Kangaparambil, S., Richter, M., Hassfurth, L., Dorner-Kirchner, M., Paulus, G.G.,... Zeiler, M. (2023). Carrier envelope phase sensitivity of photoelectron circular dichroism. Physical Chemistry Chemical Physics, 25(6), 4656-4666. https://doi.org/10.1039/d2cp03077b
MLA:
Hanus, Vaclav, et al. "Carrier envelope phase sensitivity of photoelectron circular dichroism." Physical Chemistry Chemical Physics 25.6 (2023): 4656-4666.
BibTeX: Download