Carrier envelope phase sensitivity of photoelectron circular dichroism

Hanus V, Kangaparambil S, Richter M, Hassfurth L, Dorner-Kirchner M, Paulus GG, Xie X, Baltuska A, Gräfe S, Zeiler M (2023)

Publication Type: Journal article

Publication year: 2023

Journal

Physical Chemistry Chemical Physics Royal Society of Chemistry

Book Volume: 25

Pages Range: 4656-4666

Journal Issue: 6

DOI: 10.1039/d2cp03077b

Abstract

We report on a combined experimental and numerical study of photoelectron circular dichroism (PECD) induced by intense few-cycle laser pulses, using methyloxirane as the molecular example. Our experiments reveal a remarkably pronounced sensitivity of the PECD strength of double-ionization on the carrier-envelope phase (CEP) of the laser pulses. By comparison to the simulations, which reproduce the measured CEP-dependence for specific orientations of the molecules in the lab frame, we attribute the origin of the observed CEP-dependence of PECD to the CEP-induced modulation of ionization from different areas of the wave functions of three dominant orbitals.

Involved external institutions

Technische Universität Wien / Vienna University of Technology AT Austria (AT) Friedrich-Schiller-Universität Jena DE Germany (DE)

How to cite

APA:

Hanus, V., Kangaparambil, S., Richter, M., Hassfurth, L., Dorner-Kirchner, M., Paulus, G.G.,... Zeiler, M. (2023). Carrier envelope phase sensitivity of photoelectron circular dichroism. Physical Chemistry Chemical Physics, 25(6), 4656-4666. https://dx.doi.org/10.1039/d2cp03077b

MLA:

Hanus, Vaclav, et al. "Carrier envelope phase sensitivity of photoelectron circular dichroism." Physical Chemistry Chemical Physics 25.6 (2023): 4656-4666.

BibTeX: Download