Solid state interdigitated Sb(2)S(3)based TiO(2)nanotube solar cells

Büttner P, Döhler D, Korenko S, Moehrlein S, Bochmann S, Vogel N, Minguez-Bacho I, Bachmann J (2020)


Publication Type: Journal article

Publication year: 2020

Journal

Book Volume: 10

Pages Range: 28225-28231

Journal Issue: 47

DOI: 10.1039/d0ra04123h

Abstract

TiO(2)nanotubes generated by anodization of metallic titanium sputter-coated on indium tin oxide (ITO) substrates are used as a conductive scaffold for all solid-state Sb2S3-sensitized extremely thin absorber (ETA) solar cells. A blocking layer of TiO(2)placed between Ti and ITO in combination with optimized Ti deposition and anodization conditions enables the formation of crack-free layers of straight, cylindrical TiO(2)nanotubes of tunable length and diameter. ALD (atomic layer deposition) is subsequently used to coat this substrate conformally with a highly pure Sb(2)S(3)light absorber layer under an inert atmosphere. The high absorption coefficient of Sb(2)S(3)as compared to molecular dyes allows for the utilization of very short nanotubes, which facilitates the infiltration of the organic hole transport material and formation of a p-i-n heterojunction in an interdigitated and tunable geometry. We investigate the influence of nanotube length and of the absorber thickness to enhance the photocurrent value to twice that of planar reference structures.

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How to cite

APA:

Büttner, P., Döhler, D., Korenko, S., Moehrlein, S., Bochmann, S., Vogel, N.,... Bachmann, J. (2020). Solid state interdigitated Sb(2)S(3)based TiO(2)nanotube solar cells. RSC Advances, 10(47), 28225-28231. https://doi.org/10.1039/d0ra04123h

MLA:

Büttner, Pascal, et al. "Solid state interdigitated Sb(2)S(3)based TiO(2)nanotube solar cells." RSC Advances 10.47 (2020): 28225-28231.

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