Dewetted Au films form a highly active photocatalytic system on TiO2 nanotube-stumps

Yoo JE, Lee K, Schmuki P (2013)


Publication Type: Journal article

Publication year: 2013

Journal

Book Volume: 34

Pages Range: 351-355

DOI: 10.1016/j.elecom.2013.07.008

Abstract

Highly ordered TiO2 nanotube stump-[TiO2 NS]-layers, prepared by anodization of Ti in HF/H3PO4 solutions, were used as a substrate for a thermal dewetting of Au thin films. Depending on the initial Au sputter-deposited layer thickness, various sizes and densities of gold nanoparticles [Aunp] could be obtained on the TiO2 NS. Under certain conditions, very homogeneously distributed Aunp (with diameters in the range of 2--15~nm) can be generated. Such Aunp/TiO2 NS combinations show a high efficiency for H2 production from H2O/EtOH solutions. A maximum H2 production efficiency could be obtained from a 2~nm thick Au layer (57.03~\textgreekml H2 for 9~h) that was dewetted to $≈$~28,000~particles/\textgreekmm2 with individual particle diameters of $≈$~5~nm.

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APA:

Yoo, J.E., Lee, K., & Schmuki, P. (2013). Dewetted Au films form a highly active photocatalytic system on TiO2 nanotube-stumps. Electrochemistry Communications, 34, 351-355. https://dx.doi.org/10.1016/j.elecom.2013.07.008

MLA:

Yoo, Jeong Eun, Kiyoung Lee, and Patrik Schmuki. "Dewetted Au films form a highly active photocatalytic system on TiO2 nanotube-stumps." Electrochemistry Communications 34 (2013): 351-355.

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