Vibrational Spectroscopy and Dynamics of Water
Perakis F, De Marco L, Shalit A, Tang F, Kann ZR, Kühne TD, Torre R, Bonn M, Nagata Y (2016)
Publication Type: Journal article, Review article
Publication year: 2016
Journal
Book Volume: 116
Pages Range: 7590-7607
Journal Issue: 13
DOI: 10.1021/acs.chemrev.5b00640
Abstract
We present an overview of recent static and time-resolved vibrational spectroscopic studies of liquid water from ambient conditions to the supercooled state, as well as of crystalline and amorphous ice forms. The structure and dynamics of the complex hydrogen-bond network formed by water molecules in the bulk and interphases are discussed, as well as the dissipation mechanism of vibrational energy throughout this network. A broad range of water investigations are addressed, from conventional infrared and Raman spectroscopy to femtosecond pump-probe, photon-echo, optical Kerr effect, sum-frequency generation, and two-dimensional infrared spectroscopic studies. Additionally, we discuss novel approaches, such as two-dimensional sum-frequency generation, three-dimensional infrared, and two-dimensional Raman terahertz spectroscopy. By comparison of the complementary aspects probed by various linear and nonlinear spectroscopic techniques, a coherent picture of water dynamics and energetics emerges. Furthermore, we outline future perspectives of vibrational spectroscopy for water researches.
Involved external institutions
Stanford National Accelerator Laboratory (SLAC)
United States (USA) (US)
Massachusetts Institute of Technology (MIT)
United States (USA) (US)
University of Zurich / Universität Zürich (UZH)
Switzerland (CH)
Peking University (PKU) / 北京大学
China (CN)
University of Wisconsin - Madison
United States (USA) (US)
Università degli Studi di Firenze / University of Florence
Italy (IT)
Max-Planck-Institut für Polymerforschung (MPI-P) / Max Planck Institute for Polymer Research
Germany (DE)
Universität Paderborn
Germany (DE)
United States (USA) (US)
Massachusetts Institute of Technology (MIT)
United States (USA) (US)
University of Zurich / Universität Zürich (UZH)
Switzerland (CH)
Peking University (PKU) / 北京大学
China (CN)
University of Wisconsin - Madison
United States (USA) (US)
Università degli Studi di Firenze / University of Florence
Italy (IT)
Max-Planck-Institut für Polymerforschung (MPI-P) / Max Planck Institute for Polymer Research
Germany (DE)
Universität Paderborn
Germany (DE)
How to cite
APA:
Perakis, F., De Marco, L., Shalit, A., Tang, F., Kann, Z.R., Kühne, T.D.,... Nagata, Y. (2016). Vibrational Spectroscopy and Dynamics of Water. Chemical Reviews, 116(13), 7590-7607. https://doi.org/10.1021/acs.chemrev.5b00640
MLA:
Perakis, Fivos, et al. "Vibrational Spectroscopy and Dynamics of Water." Chemical Reviews 116.13 (2016): 7590-7607.
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