Analyzing the efficiency, stability and cost potential for fullerene-free organic photovoltaics in one figure of merit

Beitrag in einer Fachzeitschrift
(Originalarbeit)


Details zur Publikation

Autorinnen und Autoren: Li N, Mcculloch I, Brabec C
Zeitschrift: Energy and Environmental Science
Verlag: Royal Society of Chemistry
Jahr der Veröffentlichung: 2018
Band: 11
Heftnummer: 6
Seitenbereich: 1355-1361
ISSN: 1754-5692
Sprache: Englisch


Abstract

The power conversion efficiencies (PCEs) of solution-processed organic
photovoltaic (OPV) devices continue increasing towards the 15%
milestone. Recently-emerging non-fullerene acceptors (NFAs) have
significantly accelerated this development. Most of the efficiency
analyses performed previously are based on a fullerene acceptor without
considering its contribution to the enhancement of photo-absorption and
PCE. Moreover, the stability and cost potential of OPV devices are usually not discussed, which sometimes makes the efficiency prediction less representative for broad interest. In this work, we effectively combine the prediction of efficiencies with experimentally determined stability data to analyze and predict the commercial potential of a NFA-based OPV product. Assuming that NFAs dominate the blend near IR absorption, the efficiency
limit of OPV devices is predicted to be close to 20% and is found to be
insensitive to the donor bandgap. With the excellent photo-stability
observed for state-of-the-art NFA-based OPV devices, it is suggested
that the corresponding customized donors with promising processing
properties, excellent environmental stability and low synthesis complexity be designed as realistic material pairs for large-scale production and commercialization.


FAU-Autorinnen und Autoren / FAU-Herausgeberinnen und Herausgeber

Brabec, Christoph Prof. Dr.
Lehrstuhl für Werkstoffwissenschaften (Materialien der Elektronik und der Energietechnologie)
Li, Ning Dr.-Ing.
Lehrstuhl für Werkstoffwissenschaften (Materialien der Elektronik und der Energietechnologie)


Einrichtungen weiterer Autorinnen und Autoren

King Abdullah University of Science and Technology (KAUST) / جامعة الملك عبد الله للعلوم و التقنية


Forschungsbereiche

Neue Materialien und Prozesse
Forschungsschwerpunkt einer Fakultät: Technische Fakultät


Zitierweisen

APA:
Li, N., Mcculloch, I., & Brabec, C. (2018). Analyzing the efficiency, stability and cost potential for fullerene-free organic photovoltaics in one figure of merit. Energy and Environmental Science, 11(6), 1355-1361. https://dx.doi.org/10.1039/c8ee00151k

MLA:
Li, Ning, Iain Mcculloch, and Christoph Brabec. "Analyzing the efficiency, stability and cost potential for fullerene-free organic photovoltaics in one figure of merit." Energy and Environmental Science 11.6 (2018): 1355-1361.

BibTeX: 

Zuletzt aktualisiert 2018-01-10 um 14:50