Molecular Mie model for second harmonic generation and sum frequency generation

Wunderlich S, Schürer B, Sauerbeck C, Peukert W, Peschel U (2011)

Publication Language: English

Publication Type: Journal article, Original article

Publication year: 2011

Journal

Physical Review B American Physical Society

Book Volume: 84

Volume: 84

Issue: 23

Journal Issue: 23

DOI: 10.1103/PhysRevB.84.235403

Abstract

A theoretical model to simulate second harmonic and sum frequency generation from stratified spherical particles of arbitrary material is presented and compared with the widely used Rayleigh-Gans-Debye approximation and to experimental results from polystyrene particles with adsorbed malachite green molecules. In this model, the nonlinear polarization is caused by individual dipoles placed in the vicinity of the sphere and is simulated on a molecular basis. This offers greater flexibility to model more sophisticated systems.

Authors with CRIS profile

Sarina Wunderlich Institut für Optik, Information und Photonik Christian Sauerbeck Lehrstuhl für Feststoff- und Grenzflächenverfahrenstechnik Wolfgang Peukert Lehrstuhl für Feststoff- und Grenzflächenverfahrenstechnik Ulf Peschel Professur für Experimentalphysik

Additional Organisation(s)

Exzellenz-Cluster Engineering of Advanced Materials

How to cite

APA:

Wunderlich, S., Schürer, B., Sauerbeck, C., Peukert, W., & Peschel, U. (2011). Molecular Mie model for second harmonic generation and sum frequency generation. Physical Review B, 84(23). https://dx.doi.org/10.1103/PhysRevB.84.235403

MLA:

Wunderlich, Sarina, et al. "Molecular Mie model for second harmonic generation and sum frequency generation." Physical Review B 84.23 (2011).

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